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Analytical chemistry aims at transforming physical and chemical properties of a sample into information about its composition. Information concerning all aspects of the molecular structure and intermolecular interactions is encoded in the vibrational spectra. The art of vibrational spectroscopy can be defined as finding the optimum approach to extracting information from the spectra of molecules and to transform it into relevant answers to analytical questions, the most simple of which are: what. and how much There are three steps which should be optimized: 1. Recording spectra in which the necessary information is encoded 2. Extracting this information 3. Decoding this information to afford solutions to analytical problems. The theory of some of the procedures discussed in the following sections are described in several books, for example by Doerffel and Eckschlager (1981), Danzer et al. (1987 a, b) and Massart et al. (1988).

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In concordance with the general construction, illustrated in 3, of coherent states on a measure space, T2 , (dx = dq d p/(2 )) in the present case, these coef cients form a nite orthogonal set in the Hilbert space L2 T2 , dq d p/(2 ) and an orthogonal basis for the N-dimensional subspace isometric to H ( ) The direct demonstration is rather cumbersome and we will omit it here Furthermore, since one is working here with a representation of the states as tempered distributions, the question of normalization is not pertinent and it is preferable to appeal to the Schur lemma and discrete Weyl Heisenberg unitary irreducible representation arguments to prove that the following resolution of the identity holds in H ( ): dq d p Z, (q, p) 2 Z, = I H (q, p)

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