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- J, Angew Chemie, 1976, 15, 630 291 Lohrenz, J C W; Woo, T K; Ziegler, T, J Am Chem Soc, 1995, 117, 12793 12800 292 Margl, P; Deng, L; Ziegler, T, J Am Chem Soc, 1999, 121, 154 162, and references therein 293 Macgregor, S A; Eisenstein, O; Whittlesey, M K; Peritz, R N, J Chem Soc Dalton Trans, 1998, 291 300 294 Ziegler, T; Tschinke, V; Fan, L; Becke, A D, J Am Chem Soc, 1989, 111, 9177 295 Wang, W; Narducci, A A; House, P G; Weitz, E, J Am Chem Soc, 1996, 118, 8654 8657 296 Han, Y; Deng, L; Ziegler, T, J Am Chem Soc, 1997, 119, 5939 5945 297 Review: Marvell, E N.

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, Thermal Electrocyclic Reactions, Academic, New York, 1980 298 Thomas IV, B E; Evanseck, J D; Houk, K N, J Am Chem Soc, 1993, 115, 4165 4169, and references therein 299 (a) Ziegenbein, W, Chem Ber, 1965, 96, 1427 (b) Goldfarb, T D; Landquist, L J, J Am Chem Soc, 1967, 89, 4588 300 Fowler, J E; Alberts, I L; Schaefer III, H F, J Am Chem Soc, 1991, 113, 4768, and references therein 301 (a) Yamazaki, H; Cvetanovic, R J, J Am Chem Soc, 1969, 91, 520 522 (b) Yamazaki, H; Cvetanovic, R J; Irwin, R S, J Am Chem Soc, 1976, 98, 2198 2205 302 Ikezawa, H; Kutal, C; Yasufuku, K; Yamazaki, H, J Am Chem Soc.

z M X l (O,O, ..., = y K t x l = (O,O, ..., O ) T ;

Axial Ratio (dB)

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, 1986, 108, 1589 1594, and references therein 303 (a) Clark, K B; Leigh, W J, J Am Chem Soc, 1987, 109, 6086 (b) Leigh, W J; Zheng, K; Clark, K B, Can J Chem, 1990, 68, 1988 304 Leigh, W J; Zheng, K, J Am Chem Soc, 1991, 113, 4019; Erratum: J Am Chem Soc, 1992, 114, 796 305 Bernardi, F; Olivucci, M; Ragazos I N; Robb, M A, J Am Chem Soc, 1992, 114, 2752 2754 306 Trulson, M O; Dollinger, G D; Mathies, R A, J Am Chem Soc, 1987, 109, 586 587 307 Martin, H-D; Urbanek, T; Pfohler, P; Walsh, R, J Chem Soc Chem Commun, 1985, 964 965..

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with' -' for positive k, '+' for negative k and the last term absent if k = O. If this rescaling is used, then (except in the k = 0 case) one loses the freedom to set a = 1 at the present time, as will be used in Section 5.3, In effect, what one is doing is choosing to measure comoving distances in units of the so-called curvature scale, which is the scale on which the effects of curved space must be included, rather than in astronomical units such as megaparsecs. In this book I will not rescale k to one of these three discrete values. though most of the time I will be specializing to k = 0 anyway.

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Even in this case, traditionally, a logarithmic form is used [Equation (9)] to treat kinetic data. The intercept of the linear plot (Figure 3) gives the value of k0 and the slope the value of ZAZB, and this is very useful information for ionic reactions to discriminate between kinetically equivalent mechanisms: log kobs = log k0 + 2aZA ZB I 1+ I (9)

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Figure B-4: This dialog box forces Photoshop to record your command, whether the program likes it or not.

15.4. 15.5.

They decouple dependency specifications from business logic, and separate crosscutting concerns. All these things are desirable in software projects of any type and/or size. The Spring framework provides generic plumbing for creating modularized applications of any kind; you are not restricted to creating web-based enterprise Java applications. Going beyond the generic plumbing discussed so far, Spring offers much, much more.

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