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Let n N be the integer closest to n Assuming that the spread W n = 1/2 n2 n 2 is small compared with n W n , we expand the energy E n in a Tay lor series in n around the centrally excited value n : En 1 1 E n + E n (n n) + E n (n n )2 + E n (n n )3 + , 2 6 (9108)



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The width of the signal monotonically increases. The average value of the g-factors (g 2.16 0.02) agrees with the g factors of isolated complexes of Cu(II), and the peak width ( H) corresponds to the total length of the spectrum. These facts suggest that the close proximity of the of copper centers are responsible for both types of the spectra. By increasing C total, the width of the singlet signal increases and con rms the existence and growth of dipole dipole interactions between copper ions. Applying Equation 1, the experimentally observed dependence of C on H is approximately linear with a slope of (9.7 2.3) 10 20 Gs cm3.56 H H0 A C (1) In addition, the contribution of copper in dipole dipole bond aggregations as it a ects C total may be estimated from the ESR data. It was shown that at a concentration exceeding 0.15 mmole/g, almost all the copper was bound as aggregates, in which the local concentration was (6.0 40.6) 1020 per cm3.55 Thus one can imagine the following distribution of copper in the grafted layer: (1) isolated complexes with an e ective distance isol 15 (Fig. 7, type I), (2) part r of the copper is in cluster-like aggregations with raggr 7 , in which the complexes





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where each prime on E n denotes a derivative These derivatives de ne distinct time scales [120], namely, the classical period T cl = 2 /|E n |; the revival time t rev = 2 / 1 |E n |; the superrevival time t sr = 2 / 1 |E n |; and so on Inserting this expan 2 6 sion into the evolution factor e iE n t/ of (9106) allows us to understand the possible occurrence of a quasiperiodic revival structure of the wave packet (9106) according to the weighting probability n |c n |2 In the present case, we have En = 2ma 2 n(n + ) = 2ma 2 n n ( + ) + (2 + )(n n ) + (n n )2 (9109) n

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So the rst characteristic time is the classical period T cl = 2 2ma 2 2 ma 2 = , 2 2 + n ( + ) n 2 (9110)

which should be compared with the actual classical (Bohr Sommerfeld) counterpart deduced from (911) and (914), T = A + a mV 0 [ 2 ma 2 ( 1) + ( 1)] (9111)

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The second characteristic time is the revival time t rev = 4 ma 2 = (2 + )T cl n (9112)

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There is no superrevival time here, because the energy is a quadratic function of n With these de nitions, the wave packet (9106) reads in the present situation (up to a global phase factor) | (t) =

(9113)

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