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Carbocation addition involves the use of vacant orbitals of the cabocation, while anionic propagation requires the use of antibonding orbitals, since all bonding orbitals on both monomer and carbanion are lled. The calculation of kp and the corresponding activation parameter Ep and A proceeds in p a reasonably straightforward manner for polymerizations in solvents of low polarity (no higher than dioxane). However, anomolous behavior is observed for polymerizations in solvents which are better solvating media than dioxane. kp is observed to increase with decreasing temperature in some systems, leading to negative activation energies. The activation energy for propagation by polystyryl sodium ion pairs in tetrahydrofuran is 6.2 kJ mol 1 over the temperature range 80 to 25 C [Shimomura et al., 1967a,b]. Ep for poly(a-methylstyryl) sodium in THF is 8.8 kJ mol 1 over the range 25 to 5 C [Hui and Ong, 1976]. 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